Sedimentation rate of settleable particulate matter in Santiago city, Chile
Verónica Morales-Casa
Departamento de Ingeniería Química y Bioprocesos, Facultad de Ingeniería, Pontificia Universidad Católica de Chile, Santiago, Chile
Center of Applied Ecology & Sustainability (CAPES UC), Pontificia Universidad Católica de Chile, Santiago, Chile
Search for more papers by this authorCorresponding Author
Francisco Barraza
Instituto de Geografía, Pontificia Universidad Católica de Chile, Santiago, Chile
School of Geography, University of Otago, Dunedin, New Zealand
Correspondence
Francisco Barraza, School of Geography, University of Otago, Dunedin, New Zealand.
Email: francisco@otago.ac.nz, fjbarraz@uc.cl
Search for more papers by this authorElizabeth Collante
Colegio Villa María Academy, Las Condes, Santiago, Chile
Search for more papers by this authorRosanna Ginocchio
Center of Applied Ecology & Sustainability (CAPES UC), Pontificia Universidad Católica de Chile, Santiago, Chile
Departamento de Ecosistemas y Medio Ambiente, Facultad de Agronomía e Ingeniería Forestal, Pontificia Universidad Católica de Chile, Santiago, Chile
Search for more papers by this authorHéctor Jorquera
Departamento de Ingeniería Química y Bioprocesos, Facultad de Ingeniería, Pontificia Universidad Católica de Chile, Santiago, Chile
Centro de Desarrollo Urbano Sustentable (CEDEUS), Santiago, Chile
Search for more papers by this authorFabrice Lambert
Instituto de Geografía, Pontificia Universidad Católica de Chile, Santiago, Chile
Centro de Ciencia del Clima y la Resiliencia (CR)2, Santiago, Chile
Search for more papers by this authorEsteban Ospina
Escuela Politécnica Nacional, Facultad de Ingeniería Civil y Ambiental, Quito, Ecuador
Search for more papers by this authorCésar Sáez-Navarrete
Departamento de Ingeniería Química y Bioprocesos, Facultad de Ingeniería, Pontificia Universidad Católica de Chile, Santiago, Chile
Centro UC de Energía, Pontificia Universidad Católica de Chile, Santiago, Chile
Search for more papers by this authorVerónica Morales-Casa
Departamento de Ingeniería Química y Bioprocesos, Facultad de Ingeniería, Pontificia Universidad Católica de Chile, Santiago, Chile
Center of Applied Ecology & Sustainability (CAPES UC), Pontificia Universidad Católica de Chile, Santiago, Chile
Search for more papers by this authorCorresponding Author
Francisco Barraza
Instituto de Geografía, Pontificia Universidad Católica de Chile, Santiago, Chile
School of Geography, University of Otago, Dunedin, New Zealand
Correspondence
Francisco Barraza, School of Geography, University of Otago, Dunedin, New Zealand.
Email: francisco@otago.ac.nz, fjbarraz@uc.cl
Search for more papers by this authorElizabeth Collante
Colegio Villa María Academy, Las Condes, Santiago, Chile
Search for more papers by this authorRosanna Ginocchio
Center of Applied Ecology & Sustainability (CAPES UC), Pontificia Universidad Católica de Chile, Santiago, Chile
Departamento de Ecosistemas y Medio Ambiente, Facultad de Agronomía e Ingeniería Forestal, Pontificia Universidad Católica de Chile, Santiago, Chile
Search for more papers by this authorHéctor Jorquera
Departamento de Ingeniería Química y Bioprocesos, Facultad de Ingeniería, Pontificia Universidad Católica de Chile, Santiago, Chile
Centro de Desarrollo Urbano Sustentable (CEDEUS), Santiago, Chile
Search for more papers by this authorFabrice Lambert
Instituto de Geografía, Pontificia Universidad Católica de Chile, Santiago, Chile
Centro de Ciencia del Clima y la Resiliencia (CR)2, Santiago, Chile
Search for more papers by this authorEsteban Ospina
Escuela Politécnica Nacional, Facultad de Ingeniería Civil y Ambiental, Quito, Ecuador
Search for more papers by this authorCésar Sáez-Navarrete
Departamento de Ingeniería Química y Bioprocesos, Facultad de Ingeniería, Pontificia Universidad Católica de Chile, Santiago, Chile
Centro UC de Energía, Pontificia Universidad Católica de Chile, Santiago, Chile
Search for more papers by this authorAbstract
Settleable particulate matter (SPM) is an atmospheric pollutant harmful to human health and the environment in high concentrations. Despite this fact, no up-to-date information on SPM levels exists for the capital of Chile, Santiago (7 million inhabitants). To address this knowledge gap, SPM sedimentation rates, including soluble and insoluble components, were measured at three different urban sites from July to November of 2016. We compare the measurements with ambient and meteorological information, as well as urban typology settings.
Our results indicate SPM deposition rates between 2.5 and 3.9 g/(m2·30 days). Only one site exceeded the national limit of 4.5 g/(m2·30 days), but we found an increasing trend in all three sites. SPM and its insoluble sedimentation rates increased during warm and dry months and presented significant correlations with meteorological parameters. The highest sedimentation rates were measured at the location with the least permeable surfaces and the lowest green spaces, while the lowest sedimentation rates were found in the sites with abundant green spaces and permeable soil. No significant differences were detected in the soluble components.
Our results suggest that SPM levels in Santiago are close to the national limit and may increase with climate change and urban expansion.
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REFERENCES
- Alahmr, F. O. M., Othman, M., Abd Wahid, N. B., Halim, A. B., & Latif1, M. T. (2012). Compositions of dust fall around semi-urban areas in Malaysia. Aerosol and Air Quality Research, 12, 629–642.
- ASTM International. (2010). Standard test method for collection and measurement of dustfall (settleable particulate matter) - D1739 − 98 (Reapproved 2010). Pensilvania, PA: Author.
- Balasubramanian, R., Victor, T., & Begum, R. (1999). Impact of biomass burning on rainwater acidity and composition in Singapore. Journal of Geophysical Research: Atmospheres, 104(D21), 26881–26890.
- Barraza, F., Lambert, F., Jorquera, H., & Villalobos, A. M., & Gallardo, L. (2017). Temporal evolution of main ambient PM2.5 sources in Santiago, Chile, from 1998 to 2012. Atmospheric Chemistry and Physics, 17, 10093–10107.
- Boisier, J. P., Rondanelli, R., Garreaud, R., & Muñoz, F. (2016). Anthropogenic and natural contributions to the southeast pacific precipitation decline and recent megadrought in Central Chile. Geophysical Research Letters, 43(1), 413–421.
- Cattle, S. R., McTainsh, G. H., & Wagner, S. (2002). Aeolian dust contributions to soil of the Namoi Valley, northern NSW, Australia. Catena, 47(3), 245–264.
- Centro Nacional Del Medio Ambiente de Chile. (2013). Evaluación de Exposición Ambiental a Sustancias Potencialmente Contaminantes Presentes En El Aire, Comunas de Concón, Puchuncaví, Quintero. Santiago, Chile: Author. http://www.cenma.cl/Pagina%20web-LQA/5-Estudios%20Ambientales/Isel-informe%20puchuncavi%2012%20septiembre.pdf.
- Chabas, A., Gentaz, L., Lombardo, T., Sinegre, R., Falcone, R., Veritàc, M., & Cachier, H. (2010). Wet and dry atmospheric deposition on TiO2 coated glass. Environmental Pollution, 158(12), 3507–3512.
- Centro Mario Molina-Chile. (2011). Análisis de Tendencia Para Material Particulado En La Región Metropolitana (2008-2010). Santiago, Chile: Author. http://metadatos.mma.gob.cl/sinia/articles-53335_Analisis_Tendencia_MP_RM_CMMC_2011.pdf.
- Center for Climate and Resilience Research (CR)2. (2015). Report to the nation. The 2010–2015 mega-drought: A lesson for the future. November 2015. Santiago, Chile. Retrieved from www.cr2.cl/megasequia
- Garcia-Chevesich, P., Alvarado, S., Neary, D., Valdes, R., Valdes, J., Aguirre, J., … Olivares, C. (2014). Respiratory Disease and particulate air pollution in Santiago Chile: Contribution of erosion particles from fine sediments. Environmental Pollution, 187, 202–205.
- Gulsona, B., Davisa, J. J., Mizon, K. J., & Bawden-Smith, J. (1995). Sources of lead in soil and dust and the use of dust fallout as a sampling medium. Science of the Total Environment, 166, 245–262.
- Gurugubelli, B., Pervez, S., & Tiwari, S. (2013). Characterization and spatiotemporal variation of urban ambient dust fallout in Central India. Aerosol and Air Quality Research, 13(1), 83–96.
- Guvenç, N., Alagha, O., & Tuncel, G. (2003). Investigation of soil multi-element composition in Antalya, Turkey. Environment international, 29, 631–640.
- Instituto Nacional de Estadísticas. (2020). Encuestas anuales de vehículos en circulación 2001–2018. Santiago, Chile. Retrieved from https://www.ine.cl/estadisticas/economia/transporte-y-comunicaciones/permiso-de-circulacion
- Machado, M., Meri-Santos, J., Reisen, V. A., Costa-Reis, N., Mavroidisc, I., & Lima, A. T. (2018). A new methodology to derive settleable particulate matter guidelines to assist policy-makers on reducing public nuisance. Atmospheric Environment, 182, 242–251.
- Malakootian, M., Ghiasseddin, M., Akbari, H., & Jaafarzadeh-Haghighi, N. A. (2013). Urban dust fall concentration and its properties in Kerman City, Iran. Health Scope, 1(4), 192–198.
10.17795/jhealthscope-8507 Google Scholar
- Ministerio de Agricultura. (1992). Decreto 4 Eexento. Normas de Calidad Del Aire Para Material Particulado Sedimentable En La Cuenca Del Rio Huasco III Región. Chile. Retrieved from https://www.leychile.cl/Navegar?idNorma=95904&idVersion=1992-05-26
- Ministerio de Salud. (2012). Estudio de Saturación Lima Metropolitana y Callao Año 2011. Lima, Peru. Retrieved from https://sinia.minam.gob.pe/documentos/estudio-saturacion-lima-metropolitana-callao-ano-2011
- Ministerio Del Medio Ambiente. (2016). Antofagasta: Presentan Resultados Parciales Del Monitoreo de Material Particulado Sedimentable (MPS). Retrieved from https://mma.gob.cl/antofagasta-presentan-resultados-parciales-del-monitoreo-de-material-particulado-sedimentable-mps/
- Moreno, F., Gramsch, E., Oyola, P., & Rubio, M. A. (2010). Modification in the Soil and traffic-related sources of particle matter between 1998 and 2007 in Santiago de Chile. Journal of the Air & Waste Management Association, 60(12), 1410–1421.
- Municipalidad de Cuenca (2015). Informe de Calidad Del Aire 2015- EMOV EP. Ecuador.
- Naddafi, K., Nabizadeh, R., Soltanianzadeh, Z., & Ehrampoosh, M. H. (2006). Evaluation of dustfall in the air of Yazd. Iranian Journal of Environmental Health Science & Engineering, 3(3), 161–168.
- Norela, S., Norfatihah, M. Z., Maimon, A., & Ismail, B. S. (2009). Wet deposition in the residential area of the Nilai Industrial Park in Negeri Sembilan, Malaysia. World Applied Sciences Journal, 7(2), 170–179.
- Nriagu, J. (1989). A global assessment of natural sources of atmospheric trace metals. Nature, 338, 47–49.
- Pandey, S. K., Tripathi, B. D., & Mishra, V. Q. (2008). Dust deposition in a sub-tropical opencast coalmine area, India. Journal of Environmental Management, 86(1), 132–138.
- Ramsperger, B., Peinemann, N., & Stahr, K. (1998). Deposition rates and characteristics of aeolian dust in the semi-arid and sub-humid regions of the Argentinean Pampa. Journal of Arid Environments, 39(3), 467–476.
- Reheis, M. C. (2006). A 16-year record of eolian dust in southern Nevada and California, USA: Controls on dust generation and accumulation. Journal of Arid Environments, 67(3), 487–520.
- Rodhe, H., Dentener, F., & Schulz, M. (2002). The global distribution of acidifying wet deposition. Environmental Science & Technology, 36(20), 4382–4388.
- Sánchez Bisquert, D., Peñas-Castejón, J. M., & García-Fernández, G. (2017). The impact of atmospheric dust deposition and trace elements levels on the villages surrounding the former mining areas in a semi-arid environment (SE Spain). Atmospheric Environment, 152, 256–269.
- Sezgin, N., Ozcan, H. K., Demir, G., Nemlioglu, D., & Bayat, C. (2004). Determination of heavy metal concentrations in street dusts in Istanbul E-5 Highway. Environment International, 29, 979–985.
- Sharma, A., Singh, S., & Kulshrestha, U. C. (2017). Determination of urban dust signatures through chemical and mineralogical characterization of atmospheric dustfall in East Delhi (India). Journal of Indian Geophysical Union, 21(2), 140–147.
- Sharma, P., Rolle, M., Kocar, B., & Fendorf, S., & Kappler, A. (2011). Influence of natural organic matter on as transport and retention. Environmental Science & Technology, 45(2), 546–553.
- Sharma, R. M., Agrawal, M., & MarshalL, F. M. (2008). Atmospheric deposition of heavy metals (Cu, Zn, Cd and Pb) in Varanasi City, India. Environmental Monitoring and Assessment, 142(1–3), 269–278.
- Trujillo-gonzález, J. M., Torres-Mora, M. A., Keesstra, S., Brevik, E. C., & Jiménez-Ballesta, R. (2016). Heavy metal accumulation related to population density in road dust samples taken from urban sites under different land uses. Science of the Total Environment, 553, 636–642.
- Valdés, A., Polvé, M., Munoz, M., & Toutain, J. P., & Morata, D. (2013). Geochemical features of aerosols in Santiago de Chile from time series analysis. Environmental Earth Sciences, 69(6), 2073–2090.
- Vallack, H. W., & Shillito, D. E. (1998). Suggested guidelines for deposited ambient dust. Atmospheric Environment, 32(16), 2737–2744.
- Yatin, M., Tuncel, S., Aras, N. K., Olmez, I., Aygun, S., & Tuncel, G. (2000). Atmospheric trace elements in Ankara, Turkey: 1. Factors affecting chemical composition of fine Particles. Atmospheric Environment, 34(8), 1305–1318.